Jimmy (Jack Wild) ventures to Living Island with his magical, talking flute, Freddy. Once there, he befriends many of the island's inhabitants, but the evil Witchiepoo (Billie Hayes) is determined to steal Freddy the flute away from the boy to impress the visiting Witches' Council and win the Witch of the Year Award.
Jimmy
Witchiepoo
Boss Witch
Witch Hazel (as Mama Cass)
H. R. Pufnstuf / Henrich Rat / Living Island Boat / Orville Pelican / Polka-Dotted Horse / Stupid Bat / West Wind (voice) (as Al Melvin)
Dr. Blinky / Ludicrous Lion / Seymore Spider / Various (voice)
Freddy the Flute / Googy Gopher / Orson Vulture (voice)
H.R. Pufnstuf
Googy Gopher / Orville Pelican
Seymore Spider / Clang
Miss Flick
Shirley Pufnstuf
Polkadotted Horse
Dr. Blinky / Ludicrous Lion
Witch Way
Witch
Orson / Cling / Various Characters
Alarm Clock
Dowager Tree / Granddaughter Clock (voice)
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